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Discovery of Charge Order and Time-Reversal Symmetry-Breaking in the Kagome Superconductor YRu$_{3}$Si$_{2}$

22 Jul 2025, 14:20
20m
Contributed Oral Magnetism Oral Contributions

Speaker

Petr Král (PSI Center for Neutron and Muon Sciences)

Description

We report the discovery of a remarkably rich phase diagram in the kagome superconductor YRu$_{3}$Si$_{2}$, uncovered through a unique combination of muon spin rotation, magnetotransport, X-ray diffraction, and density functional theory calculations. Our study reveals the emergence of a charge-ordered state with a propagation vector of (1/2, 0, 0), setting a record onset temperature of 800 K for such order in a kagome system and for quantum materials more broadly. In addition, we observe time-reversal symmetry breaking below $T_{2}^{*}$ ${\simeq}$ 30 K and field-induced magnetism below $T_{1}^{*}$ ${\simeq}$ 80 K, indicating the presence of a hidden magnetic state. These transitions are mirrored in the magnetoresistance data, which show a clear onset at 100 K and a pronounced increase below 30 K, ultimately reaching a maximum magnetoresistance of 45${\%}$. Band structure calculations identify two van Hove singularities near the Fermi level, one of which resides within a flat band, suggesting a strong interplay between electronic correlations and emergent orders. At low temperatures, we find bulk superconductivity below $T_{\rm c}$ = 3.4 K, characterized by a two-gap (s+s)-wave or anisotropic s-wave pairing symmetry. Together, our findings point to a coexistence of high-temperature charge order, tunable magnetism, and multigap superconductivity in YRu$_{3}$Si$_{2}$, positioning it as a compelling platform for exploring strongly correlated kagome physics.

Email petr.kral@psi.ch
Funding Agency Swiss National Science Foundation
Supervisors Name Zurab Guguchia
Supervisors Email zurab.guguchia@psi.ch
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Primary author

Petr Král (PSI Center for Neutron and Muon Sciences)

Co-authors

Jennifer Graham (PSI Center for Neutron and Muon Sciences CNM, Switzerland) Vahid Sazgari (PSI Center for Neutron and Muon Sciences CNM, Villigen PSI, Switzerland) Igor Plokhikh (PSI Center for Neutron and Muon Sciences CNM, Switzerland) Anastasiia Lukovkina (University of Geneva, Switzerland) Orion Gerguri (PSI Center for Neutron and Muon Sciences CNM, Switzerland) Sohel Islam (Paul Scherrer Institute) Andrin Doll (Paul Scherrer Institute) Kang Wang (University of Cambridge, United Kingdom) Malo Salamin (University of Geneva, Switzerland) Hubertus Luetkens (Paul Scherrer Institute) Rustem Khasanov (PSI Center for Neutron and Muon Sciences CNM, Switzerland) Jiaxin Yin (Southern University of Science and Technology, China) Ziqiang Wang (Boston College, USA) Bartomeu Monserrat (University of Cambridge, United Kingdom) Dariusz Gawryluk (PSI Center for Neutron and Muon Sciences CNM, Switzerland) Fabian von Rohr (University of Geneva) Sun-Woo Kim (University of Cambridge, United Kingdom) Zurab Guguchia (PSI Center for Neutron and Muon Sciences, Switzerland)

Presentation materials