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Muon-Induced X-ray Emission (MIXE) at PSI: Technique and Applications

22 Jul 2025, 15:20
20m
Contributed Oral Muonic X-rays Oral Contributions

Speaker

Michael Heiss (Paul Scherrer Institut)

Description

Muon-Induced X-ray Emission (MIXE) is a non-destructive analytical technique that combines the unique properties of negative muons with high resolution gamma detectors to perform depth-resolved elemental analysis. At PSI, the Germanium Array for Non-destructive Testing (GIANT) instrument leverages a high-intensity continuous muon beam (15–60 MeV/c) to implant muons at tunable depths (µm to cm scale). The subsequent emission of muonic X-rays during atomic de-excitation provides element-specific fingerprints, with sensitivities at the permille level for most elements in the periodic table [1,2].

In archaeology, the technique facilitated the confirmation of the meteoritic origin of a Late Bronze Age iron arrowhead by precisely measuring the high Ni content of the bulk material [3]. The analysis of a Late Antique knob bow fibula revealed dual bronze alloys: high-Pb cast components and low-Pb forged parts, indicating advanced metallurgical tailoring [4]. In energy materials, MIXE paves the way for operando analyses of batteries, such as studying transition-metal plating on electrodes, which is critical for degradation studies [5].

References

[1] S. Biswas et al., Appl. Sci. 12(5), 2541 (2022)
[2] L. Gerchow et al., Rev. Sci. Instrum. 94, 045106 (2023)
[3] B. Hofmann et al., J. Archaeol. Sci. 157, 105827 (2023)
[4] S. Biswas et al., Herit. Sci. 11, 43 (2023)
[5] F. Quérel et al., J. Mater. Chem. A 13, 2275 (2025)

Email michael.heiss@psi.ch
Funding Agency Paul Scherrer Institut
Supervisors Name Thomas Prokscha
Supervisors Email thomas.prokscha@psi.ch
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Primary author

Michael Heiss (Paul Scherrer Institut)

Co-authors

Akira Sato (Osaka University) Alex Amato (PSI Center for Neutron and Muon Sciences CNM, Switzerland) Andreas Knecht (Paul Scherrer Institut) Angela Papa (Paul Scherrer Institute) Arndt Remhof (Swiss Federal Laboratories for Materials Science and Technology) Beda Hoffmann (Naturhistorisches Museum Bern) Carlos Vigo (Paul Scherrer Institut) Charles Mielke III (PSI Center for Neutron and Muon Sciences CNM, Switzerland) Chennan Wang Corsin Battaglia (EMPA) Daniel Wiebe (University of Freiburg) Debarchan Das (Paul Scherrer Institut) Diego Ramírez García (University of Freiburg) Edouard Quérel (EMPA) Fabian Hotz (PSI Center for Neutron and Muon Sciences CNM, 5232 Villigen PSI, Switzerland) Frank Gfeller (Naturhistorisches Museum Bern) Frederik Wauters (Johannes Gutenberg Universität Mainz) Gian Müller (EMPA) Gianluca Janka (PSI) Herbert Hess (Universität zu Köln) Hubertus Luetkens (Paul Scherrer Institute) I.-Huan Chiu (Osaka University) Isabel Megatli-Niebel (Augusta Raurica) Issa Briki (Paul Scherrer Institute) Katharina von Schoeler (Paul Scherrer Institut) Kazuhiko Ninomiya (Hiroshima University) Lars Gerchow (Paul Scherrer Institut) Lilian Raselli (Augusta Raurica) Marc Schumann (University of Freiburg) Matthias Elender (Paul Scherrer Institut) Maxime Lamotte (Paul Scherrer Institute) Megumi Niikura (RIKEN Nishina Center for Accelerator Based Science) Michael Seidlitz (Universität zu Köln) Narongrit Ritjoho (Suranaree University of Technology) Nathal Severijns (KU Leuven) Nigel Warr (Universität zu Köln) Nilesh Deokar (Johannes Gutenberg Universität Mainz) Peter Reiter (Universität zu Köln) Pierre Lanari (University of Bern) Qing Wang (EMPA) Ronald Simke (Augusta Raurica) Rustem Khasanov Ryo Asakura (EMPA) Sabine Bolliger Schreyer (Bernisches Historisches Museum) Sayani Biswas (ISIS Neutron and Muon Facility) Sebastian Lindemann (University of Freiburg) Shunsuke Asari (Osaka University) Stergiani Marina Vogiatzi (KU Leuven) Thomas Elias Cocolios (KU Leuven) Thomas Prokscha (Paul Scherrer Institute) Toni Shiroka (Paul Scherrer Institut & ETH Zurich, Switzerland) Xiao Zhao (Paul Scherrer Institute) Zurab Guguchia (PSI Center for Neutron and Muon Sciences, Switzerland)

Presentation materials