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Microscopic Evidence of Field-Induced Critical Spin-Liquid State in a Metallic Frustrated Compound

Not scheduled
20m
Poster Presentation Magnetism Poster session 2

Speaker

Mr Ishant Ishant (Shiv Nadar Institution of Eminence, Greater Noida, Delhi-NCR)

Description

A field-induced quantum spin liquid (QSL) state is an extraordinary phenomenon, hitherto unobserved in metallic frustrated compounds. CePdAl (CPA), a magnetically frustrated metallic compound with a kagome lattice, presents a unique opportunity to explore this phenomenon~\cite{Kitazawa1994}. Recent bulk measurements have revealed intriguing magnetic states in CPA when a magnetic field is applied along the crystallographic c-axis~\cite{Lucas2017}. However, the nature of these field-induced states, potentially including a QSL state, remains unclear due to the lack of microscopic investigation. To elucidate these field-induced states, we employed the transverse-field muon spin relaxation/rotation (TF-$\mu$SR) technique, applying various magnetic fields parallel to the c-axis in single-crystalline CePdAl over a broad temperature range (100~K-100~mK). Our findings indicate that field-induced low-temperature states for fields B$\leq B_{c2}$ exhibit long-range magnetic order, whereas for B>$B_{c2}$ yield contrasting behavior. Notably, at 3.75 T, near a critical field $B_{c2}$, our results provide evidence of a critical spin liquid (CSL) with antiferromagnetic spin fluctuations. Furthermore, at 4.3 T, a non-Fermi liquid state is observed where frustration is absent. This comprehensive microscopic study unequivocally establishes the existence of a CSL state in a metallic frustrated system.

Email ig481@snu.edu.in
Funding Agency Shiv Nadar Institution of Eminence, Greater Noida, Delhi-NCR
Supervisors Name Dr. Mayukh Majumder
Supervisors Email mayukh.majumder@snu.edu.in
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Primary author

Mr Ishant Ishant (Shiv Nadar Institution of Eminence, Greater Noida, Delhi-NCR)

Co-authors

Dr Mayukh Majumder (Shiv Nadar Institution of Eminence, Greater Noida, Delhi-NCR) Prof. Oliver Stockert (Max Planck Institute for Chemical Physics of Solids, Dresden, Germany) Dr Veronika Fritsch (Experimental Physics VI, Center for Electronic Correlations and Magnetism, University of Augsburg, 86159 Augsburg, Germany) Dr Zurab Guguchia (Laboratory for Muon-Spin Spectroscopy, Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland)

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