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Probing Spin Dynamics in Rare-Earth Triangular Lattices YbZn$_2$GaO$_5$ and NdMgAl$_{11}$O$_{19}$

23 Jul 2025, 09:20
20m
Contributed Oral Magnetism Oral Contributions

Speaker

Hank Wu (University of Oxford)

Description

A quantum spin liquid (QSL) is a long-sought magnetic state in which strong quantum fluctuations prevent magnetic ordering, allowing spin dynamics to persist at very low temperatures. Rare-earth triangular lattice compounds have proven to be a particularly promising platform to study spin liquid behaviours due to their localised f-orbitals and inherent geometric frustration. We present $\mu$SR studies on two such compounds, YbZn$_2$GaO$_5$ and NdMgAl$_{11}$O$_{19}$, both of which exhibit both the absence of magnetic ordering and evidence of persistent dynamics down to milli-Kelvin temperatures, as shown by our $\mu$SR measurements. In YbZn$_2$GaO$_5$, the spin dynamics display a field dependence consistent with a U1A01 Dirac QSL ground state [1]. In NdMgAl$_{11}$O$_{19}$, the strong crystalline anisotropy facilitates the quantum tunneling of Ising spins and AC susceptibility measurements reveal behaviour reminiscent of spin ice pyrochlore compounds [2]. These findings highlight the potential for rare-earth triangular lattices to serve as a versatile platform for realising and studying exotic quantum magnetic states.

[1] H. C. H. Wu, F. L. Pratt, B. M. Huddart, D. Chatterjee, P. A. Goddard, J. Singleton, D. Prabhakaran, S. J. Blundell, arXiv:2502.00130.
[2] J. Snyder, J. S. Slusky, R. J. Cava, and P. Schiffer, Nature 413, 48 (2001).

Email hank.wu@physics.ox.ac.uk
Funding Agency UKRI
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Primary author

Hank Wu (University of Oxford)

Co-authors

Dr Benjamin Huddart (University of Oxford) Dharmalingham Prabhakaran (University of Oxford) Dr Dipranjan Chatterjee (University of Oxford) Francis Pratt (ISIS) Prof. John Singleton (Los Alamos National Laboratory) Prof. Paul Goddard (Warwick University) Stephen Blundell (University of Oxford)

Presentation materials