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Field-Orientation-Dependent Magnetic Phases in GdRu$_2$Si$_2$ Probed with Muon-Spin Spectroscopy

23 Jul 2025, 11:20
20m
Contributed Oral Magnetism Oral Contributions

Speaker

Dr Benjamin Huddart (University of Oxford)

Description

Centrosymmetric GdRu$_2$Si$_2$ exhibits a variety of multi-$Q$ magnetic states as a function of temperature and applied magnetic field, including a square skyrmion-lattice phase. The material’s behaviour is strongly dependent on the direction of the applied field, with different phase diagrams resulting for fields applied parallel or perpendicular to the crystallographic $c$ axis. Using transverse-field $\mu$SR with fields applied along either the [001] or [100] crystallographic directions, we distinguish between the magnetic phases in this system via their distinct muon response, providing additional evidence for the skyrmion and meron-lattice phases, while also suggesting the existence of RKKY-driven muon hyperfine coupling. Zero-field $\mu$SR provides clear evidence for a transition between two distinct magnetically ordered phases at 39 K [1].

We will also discuss novel techniques related to the computation of muon stopping sites using density functional theory (DFT), that were crucial to our analysis in this study. Notably, by considering the energy barriers for moving between muon sites, and accounting for the zero-point energy of the muon, we were able to determine that there is only a single stable crystallographically distinct site. This muon site was confirmed experimentally, using angle-dependent measurements of the muon Knight shift.

Muon sites in GdRu$_2$Si$_2$.

  1. B.M. Huddart et al., Phys. Rev. B 111, 054440 (2025).
Email benjamin.huddart@physics.ox.ac.uk
Funding Agency EPSRC (UK), UK Research and Innovation (UKRI)
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Primary author

Dr Benjamin Huddart (University of Oxford)

Co-authors

Alberto Hern ́andez-Meli ́an (University of Southampton) George Wood (ISIS) Daniel Mayoh (University of Warwick) Dr Matjaž Gomilšek (Jožef Stefan Institute & Faculty of Mathematics and Physics, University of Ljubljana) Zurab Guguchia (PSI Center for Neutron and Muon Sciences, Switzerland) Chennan Wang Thomas Hicken (Paul Scherrer Institute) Stephen Blundell (University of Oxford) Geetha Balakrishnan (University of Warwick) Tom Lancaster (Durham University)

Presentation materials